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Conductivity noise study of the insulator-metal transition and phase coexistence in epitaxial samarium nickelate thin films

机译:外延镍酸镍薄膜中绝缘体-金属过渡和相共存的电导噪声研究

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摘要

Interaction between the lattice and the orbital degrees of freedom not only makes rare-earth nickelates unusually ``bad metal,'' but also introduces a temperature-driven insulator-metal phase transition. Here we investigate this insulator-metal phase transition in thin films of SmNiO3 using the slow time-dependent fluctuations (noise) in resistivity. The normalized magnitude of noise is found to be extremely large, being nearly eight orders of magnitude higher than thin films of common disordered metallic systems, and indicates electrical conduction via classical percolation in a spatially inhomogeneous medium. The higher-order statistics of the fluctuations indicate a strong non-Gaussian component of noise close to the transition, attributing the inhomogeneity to the coexistence of the metallic and insulating phases. Our experiment offers insight into the impact of lattice-orbital coupling on the microscopic mechanism of electron transport in the rare-earth nickelates.
机译:晶格和轨道自由度之间的相互作用不仅使稀土镍酸盐异常地成为``有害金属'',而且还引入了温度驱动的绝缘体-金属相变。在这里,我们使用电阻率随时间的缓慢波动(噪声)来研究SmNiO3薄膜中的这种绝缘体-金属相变。发现噪声的归一化量级非常大,比常见的无序金属系统的薄膜高出近八个数量级,并且表明在空间不均匀介质中通过经典渗滤的导电性。波动的高阶统计表明,靠近过渡处的噪声有很强的非高斯成分,将不均匀性归因于金属和绝缘相的共存。我们的实验提供了对晶格轨道耦合对稀土镍酸盐中电子传输的微观机理的影响的见解。

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